Coherent ultrafast polaron pair formation in a conjugated polymer at room temperature
- De Sio, A
- Sommer, E
- Troiani, F
- Rehault, J
- Maiuri, M
- Molinari, E
- Cerullo, G
- Lienau, C
Publication date
January 2016
DOI Publisher
place:345 E 47TH ST, NEW YORK, NY 10017 USAAbstract
Ultrafast 2D optical spectroscopy with 10-fs-time-resolution, complemented by density matrix simulations, show that coherent vibronic coupling accelerates polaron-pair formation and results in strongly correlated exciton and polaron-pair dynamics in polythiophene thin films at room temperature
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