Two Dimensional Antiferromagnetic Chern Insulator: NiRuCl₆

Density functional theory (DFT) and Berry curvature calculations show that quantum anomalous Hall effect (QAHE) can be realized in two-dimensional­(2D) antiferromagnetic (AFM) NiRuCl₆. The results indicate that NiRuCl₆ behaves as an AFM Chern insulator and its spin-polarized electronic structure and strong spin–orbit coupling (SOC) are responsible for the QAHE. By tuning SOC, we found that the topological property of NiRuCl₆ arises from its energy band inversion. Considering the compatibility between the AFM and insulators, AFM Chern insulator provides a new way to archive high temperature QAHE in experiments due to its different magnetic coupling mechanism from that of ferromagnetic (FM) Chern insulator