In this thesis we examine a variety of question regarding several quantum information-theoretic concepts as they manifest in the context of relativistic quantum fields. In particular, we study the qualitative and quantitative structure of entanglement (as well as more generalized quantum correlations) in field theory. Primarily we study the nature of vacuum entanglement, but consider spatial correlations in more general field states as well. We also discuss several novel aspects of particle creation phenomena, which generally go hand in hand with the presence of field entanglement. Such investigations are important from two perspectives. First, we gain enlightening new insight into the nature of quantum fields and, therefore, into the funda...