Relationships between clear-sky longwave radiation and aspects of the atmospheric hydrological cycle are quantified in models, reanalyses, and observations over the period 1980–2000. The robust sensitivity of clear-sky surface net longwave radiation (SNLc) to column-integrated water vapor (CWV) of 1–1.5 W m22 mm21 combined with the positive relationship between CWV and surface temperature (Ts) explains substantial increases in clear-sky longwave radiative cooling of the atmosphere (QLWc) to the surface over the period. Clear-sky outgoing longwave radiation (OLRc) is highly sensitive to changes in aerosol and greenhouse gas concentrations in addition to temperature and humidity. Over tropical ocean regions of mean descent,QLWc increases with...